You can but the problem is it needs to be a metered application first, so, if you setup a metering rule for WinWord.exe than this information will be collected during inventory. You can than use a query or report to display this information, now the trick is you don't actually query anything, but you tell it to display the attributes "Software Usage" you can than see start times end times etc.. An example query is shown below.
Hope that helps.
Cheers
PS: The metering information can take a few days before you can run the query below because, computers need to update their local rules to tell them the application which is to be metered. It than will start to gather this information from then on, the database is only updated once an inventory has taken place, so it depends on your inventory scheduling.
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select SMS_G_System_SoftwareUsageData.* from SMS_R_System inner join SMS_G_System_SoftwareUsageData on SMS_G_System_SoftwareUsageData.ResourceID = SMS_R_System.ResourceId
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